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My system features PFBT nanoparticles and a class of merocyanine dyes.
This method then allows systematic investigation of the effects of molecular weight and side chain regioregularity of P3HT on Tg.
In addition, both side chain and backbone Tgs are identified for P3HT, while only the backbone Tg is found for PFTBT.
Although conjugated polymer is promising for applications in stretchable electronics, no rational design exists due to the lack of characterization of the fundamental properties of conjugated polymers and their interrelationships with chemical structures and performances.
Regarding the mechanical performance, the fundamental properties include the glass transition temperature (Tg), the entanglement molecular weight (Me) and the tie chain density (ρx), which dictate the stretchability of a homopolymer in different states (i.e., glassy, semicrystalline, melt).
Furthermore, data for multiple conjugated polymers with estimated persistence lengths and plateau moduli (or Me) agree reasonably well with the previously proposed universal relationship between the dimensionless Kuhn monomer density and the dimensionless rubbery plateau modulus.